电刺激响应形状记忆聚合物复合材料的设计和驱动性能

doi:10.11896/cldb.20070243

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Abstract Compared to deformable polymer materials with single expansion, contraction, and bending changes such as hydrogels, liquid crystal elastomers, and dielectric elastomers, shape memory polymers(SMPs) can be programed into a variety of complicated shapes, and its shape change is highly complex due to the capability to remember multiple shapes, which has become a hot spot in the field of intelligent materials. SMPs refer to a class of intelligent materials that sense changes in the external environment (such as temperature, light, electricity, magnetism, pH, ions, water, etc.), respond to such changes, adjust to its own state parameters (such as shape, position, strain, stress etc.) and return to a preset state. Due to large recoverable strain, diversified shape memory effects (one-way, two-way, triple, multiple, temperature-memory and stress-memory), various stimulus modes, multiple material attributes (such as thermoplastic SMPs, thermo-setting SMPs, thermadapt SMPs and shape memory hydrogels), easy shaping, easy adjustment of response temperature, and biodegradablity, SMPs have shown extremely broad application prospects in biomedicine, smart textiles, aerospace, soft robots and flexible electronics.
In a variety of SMPs, thermally stimulated SMPs are the most intensively studied and most widely used. However, the thermal driving method requires direct heating of the material to achieve the shape memory effect, which cannot be used to drive shape recovery in the internal or external space environment, limitting its applications in the biomedical, aerospace, and flexible electronics fields. For this reason, SMPs with optical, electrical, and magnetic response, which can be remotely controlled, have been widely developed, greatly expanding the application of SMPs in shielded environments and non-contact environments. However, due to the limited penetration of light and the inability to irradiate shielded areas, the application of light-responsive SMPs is limited; for magnetically responsive SMPs, with currently very few types of materials that have a magnetic field response and a required device that specifically generates a magnetic field, its application and research are subject to certain restrictions.
Electrically stimulated SMPs has attracted intense interest of researchers owing to wide application in the emerging fields of conductive mate-rials, power sources available everywhere, artificial muscles, flexible electronics, soft robots, and sensors.In this paper, the design and preparation methods, types, conductive properties, electrical-actuated shape memory properties and applications of electrically stimulated SMP compo-sites are reviewed in detail. Finally, the problems existing in electrically stimulated materials and their future development directions are summarized.

Key words： shape memory polymer composites electrically stimulated response conductive filler

Published: 25 March 2022 Online: 2022-03-21

CLC number:

O631.2

Fund:National Natural Science Foundation of China (21777065), Natural Science Foundation of Shandong Province (ZR2020QE092, ZR2020KE002),Youth Innovation Project for Colleges of Shandong Province (2019KJA021), and 2020 College Studentś Innovation and Entrepreneurship Training Program (S202010452027).

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	LI Xingjian
	HOU Qing
	YANG Jilong
	FAN Yufei
	CUI Qiuyue
	XU Shoufang

Cite this article:

LI Xingjian,HOU Qing,YANG Jilong, et al. Design and Driving Properties of Electrically Stimulated Shape Memory Polymer Composites[J]. Materials Reports, 2022, 36(6): 20070243-12.

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http://www.mater-rep.com/EN/10.11896/cldb.20070243 OR http://www.mater-rep.com/EN/Y2022/V36/I6/20070243

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