MATERIALS AND SUSTAINABLE DEVELOPMNT: MATERIALS REMANUFACTURING AND WASTE RECYCLING |
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Research Progress in the Preparation of High Cycling Stability and High Temperature CO2 Capture Materials from Industrial Solid Waste and Cheap Ore |
FAN Wenqi1, PAN Deng2, HUANG Liang1, WANG Qiang1
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1 College of Environmental Science and Engineering, Beijing Forestry University,Beijing 100083, China 2 Wuhan Kaidi Water Service Co., Ltd., Wuhan 430000, China |
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Abstract Aglobal consensus has been reached on the “2 ℃ climate red line”. In order to mitigate climate warming and meet the energy needs of economic development, CO2 emission reduction technologies have attracted wide attention. Among them, CO2 capture, utilization and storage (CCUS) technology is considered as the most ideal way to achieve emission reduction. CO2 capture is a necessary prerequisite for both utilization and storage of CO2. In recent years, air CO2 capture has been gradually concerned, but from the perspective of source control, CO2 capture from industrial sources is still the focus of emission reduction. At present, the industrial application of CO2 capture technology amine washing still has the problems of high cost and environmental toxicity. In contrast, solid CO2 capture materials have unique advantages in production, transportation and application. In view of the generally high temperature of industrial CO2, more and more researches are devoted to the construction of solid high-temperature CO2 adsorbents. At present, the high temperature CO2 capture of solid materials has entered the pilot-scale. In order to realize industrial application, the cost, adsorption performance and cycling stability of adsorptive materials have been paid much attention. Conventional high temperature CO2 adsorption materials, CaO and Li4SiO4, are prone to sintering after multiple cycles, resulting in a decline in adsorption performance. Although they can be modified by improving the synthesis method, element doping, surface modification and other means, there is no doubt that this will cause an increase in cost. In response, many researchers have begun to synthesize high-temperature CO2 adsorbents from industrial solid waste or cheap ore. A large number of research results show that the use of natural/waste raw materials can not only reduce the production cost of the adsorbent and realize the recycling of solid waste, but also some of the impurities in the raw materials have an important role in promoting the anti-sintering performance of the adsorbent, which is of great value for the practical application of solid high-temperature CO2 adsorbent. Based on the good application prospect of high temperature CO2 adsorbents synthesized from natural/waste raw materials, in order to facilitate the research and development of low cost and high efficiency CO2 adsorbents, this paper summarizes the research progress of the preparation of CaO and Li4SiO4 based high temperature CO2 adsorbents from industrial solid waste and cheap ore in the recent ten years. All kinds of precursors and modified materials are sorted out respectively, mainly include all kinds of ores (limestone, dolomite, kaolin, diatomite, vermiculite calcite, etc.), biomass (shell, shell, microorganism, valley, rice husk, etc.), cement building industrial waste (fly ash, calcium carbide slag, steel slag, calcium aluminate cement, papermaking white clay, construction waste, cement raw meal, waste marble powder, etc.), etc.; the synthesis conditions and modification methods of the materials are listed, such as doping modification, acid leaching, water washing, drying and calcination. Compared with CO2 adsorption conditions and properties based on constant cycle times and adsorption amount. The possible mechanisms, such as the optimization of surface aperture, the formation of pellet wear resistance, sintering resistance skeleton and the equilibrium diffusion of ions, are integrated. The advantages and disadvantages of all kinds of materials are summarized. For example, CaO based materials have wide sources and low cost, but there is a problem of degradation of adsorption performance caused by sintering due to cyclic calcination. Li4SiO4 based materials have a faster rate of absorption and desorption, but the problem of poor cycling stability and large influence by CO2 concentration remains to be solved. We hope that this paper can not only help researchers quickly understand the research status in this field, but also provide meaningful suggestions for their subsequent research work, so as to promote the industrial application of solid high-temperature CO2 adsorbent.
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Published: 26 September 2021
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Fund:Fundamental Research Funds for the Central Universities (2019JQ03015), the National Natural Science Foundation of China (U1810209), the International Science and Technology Cooperation Project of Bingtuan (2018BC002) and the Beijing Municipal Education Commission for Their Financial Support Through Innovative Transdisciplinary Program “Ecological Restoration Engineering”. |
About author:: Wenqi Fanachieved her B. S. degree in environmental engineering from Beijing Forestry University in June 2019. She is currently persuing her master’s degree at the college of Environmental Science and Engineering, Beijing Forestry University under the supervision of Prof. Wang Qiang. Her research has focused on alkali metal titanate high-temperature CO2 adsorption mate-rials. Qiang Wang, vice director, professor and doctoral supervisor of the College of Environmental Science and Engineering, Beijing Forestry University. He received his bachelor’s and master’s degrees from Harbin Institute of Technology in 2003 and 2005, and his Ph.D. from Pohang University of Technology in South Korea in 2009. He was a researcher at the Institute of Chemical and Engineering Sciences of the Singapore Research Agency from 2009 to 2011. After a year of postdoctoral research at Oxford University in UK, he joined the School of Environmental Science and Engineering of Beijing Forestry University in 2012. His main research directions include: (1) carbon dioxide capture and utilization; (2) research and development of flue gas denitration catalysts; (3) research and development of volatile organic pollutant adsorption/catalytic materials. |
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