金属有机骨架材料合成方法对氮氧化物吸附性能的影响

Abstract
Figure/Table
References
Related Citation (4)

Download:

Full Text ( PDF ) (4132KB)
Export: BibTeX | EndNote (RIS)

Abstract Metal organic framework materials have good gas adsorption performance due to their high specific surface area and porosity. Compared with traditional NOx adsorption materials, MOFs have ultra-high specific surface area and porosity, rich and diverse structures and periodicity, and good thermal and chemical stability. The synthesis methods of MOFs have been studied a lot to get a high adsorption efficiency of NOx.
The synthesis methods of MOFs mainly include hydrothermal method, solvothermal method, ultrasonic synthesis method and microwave synthesis method. The hydrothermal method has an easy operation and high crystal quality but a large crystal grains and small pore volume; The principles of the solvothermal method and the hydrothermal method are same. By adding organic solvents with different functional groups, the synthesized material can have a richer structure, larger specific surface area, and a better adsorption property on NOx than hydrothermal method. So it is also the most widely used method; the MOFs synthesized by ultrasonic synthesis method has small particle and uniform size,large specific surface area and pore volume, and good NOx adsorption property but high cost; the microwave synthesis method can accelerate the reaction process to get a smaller particle size, specific surface area and pore volume, and a high adsorption capacity for NOx, but it also has the disadvantage of high economic cost.
Therefore, we summarize the synthesis methods and modification technologies of MOFs in this article, and analyze the effects of MOFs synthesized by different methods on the adsorption of NOx, and then prospecte the development trend of MOFs for adsorbing NOx.

Key words： metal organic framework materials nitrogen oxides dry adsorbent synthesis method

Published: 16 July 2021

CLC number:

TB383

Fund:National Natural Science Fountation of China(51872265), the “13th Five-Year”Research and Development Program of China(2017YFB0310701).

About author:: Xinghui Cui received her B.E. degree in Luoyang Institute of Science and Technology in 2018. She is currently pursuing her master's degree at the School of Materials Science and Engineering,Zhengzhou University under the supervision of associate professor Chengliang Ma.Her research has focused on nitrogen oxide emission reduction technology in high temperature kilns.Chengliang Ma is a professor of Zhengzhou University, a doctoral supervisor, the director of the Institute of High Temperature Materials of Zhengzhou University, and the director of the Henan Provincial Key Laboratory of High Temperature Functional Materials. Received a Ph.D. in Materials Processing from Zhengzhou University in 2006 (supervised by Academician Xiangchong Zhong). From November 2000 to present, he has been working at the School of Materials of Zhengzhou University/Institute of High Temperature Functional Materials of Zhengzhou University,December 2018 to December 2019, as a national public visiting scholar at Wake Forest University, USA. He has published more than 50 papers in domestic and foreign academic journals, published 4 monographs, 10 achievements have been identified as internationally advanced, authorized more than 10 national patents, and presided over 3 national natural science foundation projects. The research direction is mainly high-efficiency energy-saving heat insulation materials, new refractory materials for clean steel smelting ladle, and non-oxide composite materials. Won the first Xiangchong Zhong Youth Science and Technology Award, the National Building Material Industry Technology Innovation Award, the National New Product Award, the Second Prize of Henan Science and Technology Progress Award,the Henan Provincial Department of Education Science and Technology Achievement Award, and was named the first prize of "Zhihui Zhengzhou" in 2018 Approve local talents with outstanding contributions. The paper has won the first prize of the 10th Henan Provincial Outstanding Paper in Natural Science, and the first prize of the Henan Provincial Department of Education. Independently or assist Academician Xiangchong Zhong to supervise dozens of master and doctoral students.

	Service
	E-mail this article
	Add to my bookshelf
	Add to citation manager
	E-mail Alert
	RSS
	Articles by authors
	CUI Xinghui
	WU Xiaopeng
	QI Wenhao
	XING Yiqiang
	PAN Mengbo
	DU Haoran
	MA Chengliang

Cite this article:

CUI Xinghui,WU Xiaopeng,QI Wenhao, et al. Influence of Metal Organic Framework Materials Synthesis Method on the Adsorption Performance of Nitrogen Oxides[J]. Materials Reports, 2021, 35(Z1): 121-127.

URL:

http://www.mater-rep.com/EN/ OR http://www.mater-rep.com/EN/Y2021/V35/IZ1/121

1 王宗雄, 储荣邦. 表面工程资讯, 2011, 11(2), 3.
2 Matito-Martos I, Rahbari A, Martin-Calvo A, et al. Phyical Chemistry Chemical Physics, 2018, 20(6), 4189.
3 马现奇, 高旭东, 范永斌, 等. 中国水泥, 2019(5), 78.
4 Zengel D, Koch P, Torkashvand B, et al. Angewandte Chemie International Edition, 2020, 132(34), 11423.
5 Ye B, Kim J, Lee M J, et al. Microporous and Mesoporous Materials, 2021, 310, 110588.
6 Klose W, Rincon S. Fuel, 2007, 86(1-2), 203.
7 Perdana I, Creaser D, Hrman O, et al. Journal of Catalysis, 2005, 234(1), 219.
8 李娟娟. 吸附脱除低浓度一氧化氮的研究. 硕士学位论文, 大连理工大学, 2017.
9 Li H L, Eddaoudi M, O'Keeffe M, et al. Academic Journal, 1999, 402(6759), 4.
10 郭大为, 李倩, 陈西岩, 等.石油炼制与化工, 2012, 42(2), 9.
11 Xu Q, Fang L, Fu Y, et al. Materials Letters, 2020, 264, 127402.
12 Zhao X, Wang Y, Li D S, et al. Advanced Materials, 2018, 30(37), 1705189.1.
13 Kim K C. Journal of Organometallic Chemistry, 2018, 854, 94.
14 Chavan S, Vitillo J G, Gianolio D, et al. Physical Chemistry Chemical Physics, 2012, 14(5), 1614.
15 王丽苹, 赵粒成, 兰开顺, 等. 化学通报, 2017, 80(7) , 14.
16 Glomb S, Woschko D, Makhloufi G, et al. Acs Applied Materials & Interfaces, 2017, 9(42), 37419.
17 Petit C, Levasseur B, Mendoza B, et al. Microporous and Mesoporous Materials, 2012, 154, 107.
18 Yu J. Computational evaluation of metal-organic frameworks for CO₂ capture. Ph.D.Thesis, Texas A&M University, USA, 2013.
19 Tan K, Zuluaga S, Gong Q, et al. Chemistry of Materials, 2015, 27(6), 2203.
20 Levasseur B, Petit C, Bandosz T J. ACS Applied Materials and Interfaces, 2010, 2(12), 3606.
21 Breedon M, Spencer M J S, Miura N. The Journal of Physical Chemistry C, 2013, 117(24), 12472.
22 Breedon M, Spencer M J S, Miura N. Chemical Physics Letters, 2014, 593, 61.
23 Liu Z S. Waste Management, 2008, 28(11), 2329.
24 Khan A H, Peikert K, Fröba M, et al. Microporous and Mesoporous Materials, 2015, 216, 111.
25 Meek S T, Greathouse J A, Allendorf M D. Advanced Materials, 2011, 23(2), 249.
26 Zheng N, Masel R I. Journal of the American Chemical Society, 2006, 128(38), 12394.
27 Seo Y K, Hundal G, Jang I T, et al. Microporous and Mesoporous Mate-rials, 2009, 119(1), 331.
28 Vaitsis C, Sourkouni G, Argirusis C. Ultrasonics sonochemistry, 2019, 52, 106.
29 Klimakow M, Klobes P, Thu Nemann A F, et al. Chemistry of Materials, 2010, 22(18), 5216.
30 乔萌, 牛建瑞, 钟为章, 等. 河北工业科技, 2018, 167(1), 74.
31 Chui S S Y, Lo S M F, Charmant J P H, et al. Science, 1999, 283(5405), 1148.
32 Yang S H, Sun J L, Ramirez-Cuesta A J, et al. Green Chemistry, 2012, 4(11), 887.
33 Ibarra I A, Bayliss P A, Pérez E, et al. Green Chemistry, 2012, 14(1), 117.
34 Han X, Godfrey H G W, Briggs L, et al. Nature Materials, 2018, 17(8), 691.
35 Nijem N, Bluhm H, Ng M L, et al. Chemical Communications Royal Society of Chemistry, 2014, 50(70), 10144.
36 Petit C, Bandosz T J. Dalton Transactions, 2012, 41(14), 4027.
37 Sava Gallis D F, Vogel D J, Vincent G A, et al. ACS Applied Materials and Interfaces, 2019, 11(46), 43270.
38 Gupta A, Kang S B, Harold M P. Catal. Today, 2021, 360, 411.
39 Bello E, Margarit V J, Gallego E M, et al. Microporous and Mesoporous Materials, 2020, 302, 110222.
40 Han X, Hong Y, Ma Y, et al. Journal of the American Chemical Society, 2020, 142(36), 15235.
41 Lu Z, Godfrey H G W, Da Silva I, et al. Nature Communications, 2017, 8, 14212.
42 Kyriakidou E A, Lee J, Choi J S, et al. Catal. Today, 2020, 360.
43 Li J, Han X, Zhang X, et al. Nature Chemistry, 2019, 11(12), 1085.
44 Xiang L, Blake A J, Wilson C, et al. Journal of the American Chemical Society, 2006, 128(33), 10745.
45 聂明, 陆顺, 李庆, 等.中国科学:化学, 2016, 46(4), 357.
46 Cavka J H, Jakobsen S R, Olsbye U, et al. Journal of the American Chemical Society, 2008, 130(42), 13850.
47 Ebrahim A M, Levasseur B, Bandosz T J. Langmuir, 2012, 29(1), 168.
48 Ebrahim A M, Bandosz T J. Microporous & Mesoporous Materials, 2014, 188, 149.
49 Wang Y, Ercan C, Khawajah A, et al. Aiche Journal, 2012, 58(3), 782.
50 Li B, Wen H-M, Wang H, et al. Energy & Environmental Science, 2015, 8(8), 2504.
51 Ebrahim A M, Bandosz T J. ACS Applied Materials and Interfaces, 2013, 5(21), 10565.
52 陈驰, 庞军, 韩爽, 等. 物理化学学报, 2012, 28(1), 189.
53 Wang L, Wang L, Zhao J, et al. Journal of Applied Physics, 2012, 111(11) , 112628.
54 Chae H K, Siberio-Pérez D Y, Kim J, et al. Nature, 2004, 427(6974), 523.
55 Caskey S R, Wong-Foy A G, Matzger A J. Journal of the American Che-mical Society, 2008, 130(33), 10870.
56 Tan K, Zuluaga S, Wang H, et al. Chemistry Materials, 2017, 29(10), 4227.
57 王玮, 吴云, 迟博伟. 化工设计通讯, 2016, 42(9), 32.
58 Bo X, Wheatley P S, Zhao X, et al. Journal of the American Chemical Society, 2007, 129(5), 1203.
59 侯吉聪.山东化工, 2019, 48(10), 81.
60 Petit C, Burress J, Bandosz T J. Carbon, 2011, 49(2), 563.
61 Seredych M, Bandosz T J. Journal of Physical Chemistry C, 2007, 111(43), 15596.
62 Decoste J B, Demasky T J, Katz M J, et al. New Journal of Chemistry, 2015, 39(4), 2396.
63 Katz M J, Brown Z J, Colon Y J, et al. Chemical Communications, 2013, 49(82), 9449.
64 张林建, 李芳芹, 任建兴, 等. 上海电力学院学报, 2019, 35(3), 267.
65 Thomas-Hillman I, Stevens L A, Lange M, et al. Green Chemistry, 2019, 21(18), 5039.
66 Peterson G W, Mahle J J, DeCoste J B, et al. Angewandte Chemie, 2016, 128 (21) , 6343.